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Beilstein J. Org. Chem. 2013, 9, 733–742, doi:10.3762/bjoc.9.83
Graphical Abstract
Scheme 1: Examples of selective photolysis of the azido groups.
Scheme 2: Possible photoproducts of triazide 11.
Figure 1: EPR spectra: (a) simulated spectrum for a mixture of five nitrenes with (i) S = 1, g = 2.003, DT = ...
Figure 2: UB3LYP/6-311G*+BLYP/EPRII calculated orientations of the tensors DSS and DSO in nitrenes 15–18. The...
Figure 3: Mulliken spin populations on the nitrene units and parameters DTSS in cm−1 of triplet nitrenes 12–14...
Scheme 3: Initial stages of the photolysis of triazide 11.
Figure 4: UB3LYP/6-311+G* orbital density in the LUMO of triazide 11 and CIS/6-311+G* orbital density in the ...